Resonant and nonresonant second-harmonic generation in a single cadmium sulfide nanowire
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摘要:
We experimentally investigate the resonant and nonresonant second-harmonic generation in a single cadmium sulfide (CdS) nanowire.The second-order susceptibility tensor is determined by analyzing the forward second-harmonic signals of the CdS nanowire.Our results show that (1) d33/d31 =-2.5 at a nonresonant input wave-length of 1050 nm;(2) d33/d31 =-1.9 at a resonant wavelength of 740 nm.The difference can be attributed to the polarization-dependent resonance.