Dynamical analysis of the effect of elliptically polarized laser pulses on molecular alignment and orientation
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摘要:
In this Letter,we study the molecular alignment and orientation driven by two elliptically polarized laser pulses.It is shown that the field-free molecular alignment can be achieved in a three-dimensional (3D) case,while the field-free molecular orientation is only along the x and y directions,and that the field-free alignment and orientation along different axes are related to the populations of the rotational states.It is demonstrated that changing the elliptic parameter is efficient for controlling both in-pulse and post-pulse molecular alignment and orientation.The delay time also has an influence on the field-free molecular alignment and orientation.