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High-quality Bi2?xPbxSr2CaCu2O8+δ (Bi2212) single crystals have been successfully grown by the traveling solvent floating zone technique with a wide range of Pb substitution (x=0–0.8). The samples are characterized by transmis-sion electron microscope (TEM) and measured by high resolution laser-based angle-resolved photoemission spectroscopy (ARPES) with different photon energies. A systematic evolution of the electronic structure and superstructure with Pb substitution has been revealed for the first time. The superstructure shows a significant change with Pb substitution and the incommensurate modulation vector (Q) decreases with increasing Pb substitution. In the meantime, the superstructure intensity from ARPES measurements also decreases dramatically with increasing Pb concentration. The superstructure in Bi2212 can be effectively suppressed by Pb substitution and it nearly disappears with a Pb substitution of x=0.8. We also find that the superstructure bands in ARPES measurements depend sensitively on the photon energy of lasers used;they can become even stronger than the main band when using a laser photon energy of 10.897 eV. These results provide important information on the origin of the incommensurate superstructure and its control and suppression in bismuth-based high temperature superconductors.
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篇名 Evolution of incommensurate superstructure and electronic structure with Pb substitution in (Bi2?xPbx)Sr2CaCu2O8+δ superconductors
来源期刊 中国物理B(英文版) 学科
关键词 Bi2?xPbxSr2CaCu2O8+δ superstructure electronic structure angle-resolved photoemission spec-troscopy (ARPES) modulation
年,卷(期) 2019,(7) 所属期刊栏目
研究方向 页码范围 111-120
页数 10页 分类号
字数 语种 英文
DOI 10.1088/1674-1056/28/7/077403
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Bi2?xPbxSr2CaCu2O8+δ
superstructure
electronic structure
angle-resolved photoemission spec-troscopy (ARPES)
modulation
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中国物理B(英文版)
月刊
1674-1056
11-5639/O4
北京市中关村中国科学院物理研究所内
eng
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17050
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