Thermochromic Silks for Temperature Management and Dynamic Textile Displays
Thermochromic Silks for Temperature Management and Dynamic Textile Displays
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摘要:
Silks have various advantages compared with synthetic polymer fib-ers, such as sustainability, mechanical properties, luster, as well as air and humidity permeability. However, the functionalization of silks has not yet been fully devel-oped. Functionalization techniques that retain or even improve the sustainability of silk production are required. To this end, a low-cost, effective, and scalable strategy to produce TCSs by integrating yarn-spinning and continuous dip coating technique is developed herein. TCSs with extremely long length (> 10 km), high mechanical performance (strength of 443.1 MPa, toughness of 56.0 MJ m?3, comparable with natural cocoon silk), and good interfacial bonding were developed. TCSs can be automatically woven into arbitrary fabrics, which feature super-hydrophobicity as well as rapid and programmable thermochromic responses with good cyclic perfor-mance: the response speed reached to one second and remained stable after hun-dreds of tests. Finally, applications of TCS fabrics in temperature management and dynamic textile displays are demonstrated, confirming their application potentialin smart textiles, wearable devices, flexible displays, and human–machine interfaces. Moreover, combination of the fabrication and the demonstrated applications is expected to bridge the gap between lab research and industry and accelerate the commercialization of TCSs.