Study of aerosol characteristics and sources using MAX-DOAS measurement during haze at an urban site in the Fenwei Plain

• 作者: Xiaomei Li Pinhua Xie Ang Li Jin Xu Hongmei Ren Bo Ren Yanyu Li Jie Li
• 来源期刊: 环境科学学报（英文版）
• 年，卷（期）: 2021,（9）
• 所属期刊栏目: Regular articles
• 页码范围: 1-13
• 页数: 13页
• 语种: 英文

摘要

Atmospheric aerosols have effects on atmospheric radiation assessments, global climate change, local air quality and visibility. In particular, aerosols are more likely transformed and accumulated in winter. In this paper, we used the Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) instrument to study the characteristics of aerosol type and con-tributions of PM2.5 chemical components to aerosol extinction (AE), vertical distribution of aerosols, and source. From December 30, 2018 to January 27, 2019, we conducted MAX-DOAS observations on Sanmenxia. The proportion of PM2.5 to PM10 was 69.48％-95.39％, indicating that the aerosol particles were mainlyfine particles. By analyzing the ion data and modifying Interagency Monitoring of Protected Visual Environments (IMPROVE) method, we found that nitrate was the largest contributor to AE, accounting for 31.51％, 28.98％, and 27.95％ of AE on heavily polluted, polluted, and clean days, respectively. NH4+ , OC, and SO42- were also major contributors to AE. The near-surface aerosol extinction retrieved from MAX-DOAS measurement the PM2.5 and PM10 concentrations measured by an Unmanned Aerial Vehi-cle (UAV) have the same trend in vertical distribution. AE increased about 3 times from sur-face to 500 m. With the backward trajectory of the air mass during the haze, we also found that the continuous heavy pollution was mainly caused by transport of polluted air from the northeast, then followed by local industrial emissions and other sources of emissions under continuous and steady weather conditions.