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摘要:
There are several natural materials which have evolved functional gradients,ingeniously attaining maximal efficacy from limited components.Herein,we utilized the spatiotemporal distribution of initiator acetylacetone to regulate the multienzyme poly-merization and fabricate a chitosan-polymer hydrogel.The temporal priority order of acetylacetone was higher than phenol-modified chitosan by density functional theory calculation.The acetylacetone within the gelatin could gradually diffuse spatially into the chitosan hydrogel to fabricate the composite hydrogel with gradient network structure.The gradient hydrogel possessed a transferring topography from the two-dimensional pattem.A continuously decreased modulus along with acetylacetone diffusion was confirmed by atomic force microscope-based force mapping experiment.The water-retaining ability of various regions was confirmed by low-field nuclear magnetic resonance (NMR) and thermogravimetric analysis (TG) analysis,which led to the spontaneous actuation of gradient hydrogel with maximum 1821°/h curling speed and 227° curling angle.Conse-quently,the promising gradient hydrogels could be applied as intelligent actuators and flexible robots.
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篇名 Spatiotemporally-regulated multienzymatic polymerization endows hydrogel continuous gradient and spontaneous actuation
来源期刊 中国科学:化学(英文版) 学科
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年,卷(期) 2022,(1) 所属期刊栏目 ARTICLES
研究方向 页码范围 153-161
页数 9页 分类号
字数 语种 英文
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中国科学:化学(英文版)
月刊
1674-7291
11-5839/O6
16开
北京东黄城根北街16号
1950
eng
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