Characteristics of PM2.5 pollution in Beijing after the improvement of air quality

• 作者: Xiaojuan Huang Guiqian Tang Junke Zhang Baoxian Liu Chao Liu Jin Zhang Leilei Cong Mengtian Cheng Guangxuan Yan Wenkang Gao Yinghong Wang Yuesi Wang
• 来源期刊: 环境科学学报（英文版）
• 年，卷（期）: 2021,（2）
• 页码范围: 1-10
• 页数: 10页
• 语种: 英文

摘要

Following the implementation of the strictest clean air policies to date in Beijing,the physic-ochemical characteristics and sources of PM2.5 have changed over the past few years.To improve pollution reduction policies and subsequent air quality further,it is necessary to explore the changes in PM2.5 over time.In this study,over one year(2017-2018)field study based on filter sampling(TH-150C;Wuhan Tianhong,China)was conducted in Fengtai Dis-trict,Beijing,revealed that the annual average PM2.5 concentration(64.8 ± 43.1 μg/m3)was significantly lower than in previous years and the highest PM2.5 concentration occurred in spring(84.4 ± 59.9 μg/m3).Secondary nitrate was the largest source and accounted for 25.7％of the measured PM2.5.Vehicular emission,the second largest source(17.6％),deserves more attention when considering the increase in the number of motor vehicles and its contri-bution to gaseous pollutants.In addition,the contribution from coal combustion to PM2.5 decreased significantly.During weekends,the contribution from EC and NO3-increased whereas the contributions from SO42-,OM,and trace elements decreased,compared with weekdays.During the period of residential heating,PM2.5 mass decreased by 23.1％,com-pared with non-heating period,while the contributions from coal combustion and vehicular emission,and related species increased.With the aggravation of pollution,the contribution of vehicular emission and secondary sulfate increased and then decreased,while the con-tribution of NO3-and secondary nitrate continued to increase,and accounted for 34.0％and 57.5％of the PM2.5 during the heavily polluted days,respectively.