Transparent perovskite glass-ceramics for visual optical thermometry

• 作者: Qihua Yang Lei Zhao Zhaohui Fang Ze Yang Jiangyan Cao Yiyu Cai Dacheng Zhou Xue Yu Jianbei Qiu Xuhui Xu
• 来源期刊: 稀土学报（英文版）
• 年，卷（期）: 2021,（6）
• 所属期刊栏目: ADVANCED RARE EARTH MATERIALS
• 页码范围: 712-717
• 页数: 6页
• 语种: 英文

摘要

Optical thermometers have aroused considerable attention in recent years,and the increasing demand of sensitivity for practical application encourages the investigation on developing innovative non-contact optical thermometric materials with higher sensitivity and accuracy.Perovskite quantum dots (QDs)with excellent temperature-dependence optical properties,provide a feasible approach to realizing the detection of temperature change,however,their poor high temperature thermal stability and the facile realization to obtain the production remain a daunting challenge.Herein,growing Tb3+-doped CsPbI3 QDs in situ in borosilicate glass is proposed,which ensures the phase stability,and high-efficiency florescence output of the all-inorganic perovskite as a temperature sensor.A higher absolute and rela-tive temperature sensitivity (0.0398 K-1 and 7.12％/K,respectively),along with the visible color change from orange-red to yellow-green with the increase of temperature is accomplished.Notably,the repeatable florescence intensity of Tb3+-doped CsPbI3 QDs under high temperature enables their tem-perature sensing application.