Structure, magnetic and transport properties of YMn6Sn6-xGax (0 ≤ x ≤ 0.6) compounds with a HfFe6Ge6-type
structure were investigated. It was found that the Ga substitution leads to a contraction of the unit-cell volume. A
transition from an antiferromagnetic to a ferromagnetic (or ferrimagnetic) state can be observed for samples (0.1 ≤
x ≤ 0.2) with increasing temperature. The antiferro-ferromagnetic transition for samples with x ≤ 0.2 can also be
induced by an external field. The required field is very low, and decreases with increasing Ga concentration. More
Ga concentration (x ≥ 0.3) leads to the samples being ferromagnetic in the whole temperature range below the Curie
temperature. The Ga substitution weakens the interlayer magnetic coupling between the Mn spins. Corresponding
to the metamagnetic transition, a magnetoresistance as large as 32% under a field of 5 T was observed at 5 K for the
sample with x=0.2.