With the rapid emergence of wearable devices,flexible lithium-ion batteries (LIBs) are much more needed than ever.Free-standing graphene-based composite paper electrodes with various active materials have appealed wide applications in flexible LIBs.However,due to the prone-to-restacking feature of graphene layers,a long cycle life at high current densities is rather difficult to be achieved.Herein,a unique three-dimensional (3D) hierarchically porous NiO micro-flowers/graphene paper (fNiO/GP) electrode is successfully fabricated.The resulting fNiO/GP electrode shows superior long-term cycling stability at high rates (e.g.,storage capacity of 359 mAh/g after 600 cycles at a high current density of 1 A/g).The facile 3D porous structure combines both the advantages of the graphene that is highly conductive and flexible to ensure rapid electrons/ions transfer and buffer the volume expansion of NiO during charge/discharge,and of the micro-sized NiO flowers that induces hierarchical between-layer pores ranging from nanomicro meters to promote the penetration of the electrolyte and prevent the re-stacking of graphene layers.Such structural design will inspire future manufacture of a wide range of active materials/graphene composite electrodes for high performance flexible LIBs.