Simulation Study of Passive Rod Diffusion in Active Bath:Nonmonotonic Length Dependence and Abnormal Translation-Rotation Coupling

• 作者: Rui-kai Xu Hui-jun Jiang Zhong-huai Hou
• 来源期刊: 化学物理学报（英文版）
• 年，卷（期）: 2021,（2）
• 所属期刊栏目: ARTICLE
• 页码范围: 157-164
• 页数: 8页
• 语种: 英文
• DOI: 10.1063/1674-0068/cjcp2006091

摘要

Diffusion of tracer particles in active bath has attracted extensive attention in recent years.So far,most studies have considered isotropic spherical tracer particles,while the diffusion of anisotropic particles has rarely been involved.Here we investigate the diffusion dynamics of a rigid rod tracer in a bath of active particles by using Langevin dynamics simulations in a two-dimensional space.Particular attention is paid to how the translation (rotation)diffusion coefficient DT (DR) change with the length of rod L and active strength Fa.In all cases,we find that rod exhibits superdiffusion behavior in a short time scale and returns to normal diffusion in the long time limit.Both DT and DR increase with Fa,but interestingly,a nonmonotonic dependence of DT (DR) on the rod length has been observed.We have also studied the translation-rotation coupling of rod,and interestingly,a negative translation-rotation coupling is observed,indicating that rod diffuses more slowly in the parallel direction compared to that in the perpendicular direction,a counterintuitive phenomenon that would not exist in an equilibrium counterpart system.Moreover,this anomalous (diffusion) behavior is reentrant with the increase of Fa,suggesting two competitive roles played by the active feature of bath particles.