Subsurface intercalation activating basal plane of black phosphorus for nitrogen reduction

• 作者: Xue Zhang Haitao Zhao Paul K.Chu Jiahong Wang Xue-Feng Yu
• 来源期刊: 能源化学
• 年，卷（期）: 2021,（9）
• 页码范围: 293-299
• 页数: 7页
• 语种: 英文

摘要

1.Introduction Ammonia(NH3)is not only an important chemical in many fields,but also provides a promising intermediate for energy stor-age[1,2].To produce NH3 from naturally abundant N2,the strong N≡N bond in the inert N2 molecules must be broken firstly.Elec-trochemical nitrogen reduction reaction(N2RR)under ambient conditions holds the great promise to directly produce NH3 from abundant N2 and renewable electricity in aqueous solutions[3-13].